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From
Diazotype – A Historical Copying Process
Matthias Ducci
World Journal of Chemical Education
.
2021
, 9(4), 136-143 doi:10.12691/wjce-9-4-6
Figure 1.
Structural formulae of picramic acid (left) and 2-diazo-4,6-dinitrophenol (right)
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Figure 2.
Ionic (top) and radical (bottom) C-N bond cleavage.
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Figure 3.
Sequence of photolysis and subsequent phenol formation after ionic decay of the excited singlet diazonium cation (modified according to [11])
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Figure 4.
Acidic (left), neutral (middle) and alkaline 5-ASA solution under UV light (λ = 365 nm). (Photographs: Ducci)
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Figure 5.
Equilibria of 5-ASA in aqueous solution
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Figure 6.
5-Diazosalicylic acid. (Photograph: Ducci)
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Figure 7.
Thermolysis of 5-diazosalicylic acid. The time between the two images was 1/25 s. (Photographs: Ducci)
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Figure 8.
Diazotisation of 5-ASA and formation of 5-diazosalicylic acid
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Figure 9.
Diazonium salt solution under UV light (λ = 365 nm; top: immediately after dropping the solution onto a filter paper; middle: after 5 seconds; bottom: after 45 seconds). (Photographs: Ducci)
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Figure 10.
Left: Photochemically generated image using a fern leaf under UV light. Right: The same image after prolonged irradiation with UV light (λ = 365 nm). (Photographs: Ducci)
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Figure 11.
Irradiation of the diazonium salt solution leads to the formation of gas bubbles of nitrogen. (Photograph: Ducci)
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Figure 12.
Illustration of photolytic nitrogen removal with subsequent formation of 2,5-dihydroxybenzoic acid with structural formulae
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Figure 13.
From top to bottom: Original photo (Ducci), printout as black and white image on foil, image obtained by diazotype, same image under UV light (motif: East Side Gallery Berlin/Germany)
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Figure 14.
Coupling reaction with phloroglucinol
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Figure 15.
Top: Diazotype with a red azo dye (motif: Temple of Augustus, Pula/Croatia); bottom: Foil print used.
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Figure 16.
Top: Diazotype with yellow azo dye (motif: Traditional Turkish houses in the centre of Ankara/Turkey); bottom: The same image under UV light (λ = 365 nm)
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Figure 17.
Diazotype with a mixture of a yellow and a red azo dye (motif: Giant Ferris Wheel
in the Vienna Prater/Austria)
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Figure 18.
Concurrent syntheses ((a) with 2-naphthol and (b) with resorcinol) of a red (a) and a yellow (b) azo dye, yielding the mixed colour orange in Figure 17
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Figure 19.
Diazotype with a blue azo dye (top), which takes on a reddish-brown hue at a lower pH value (outgassing of ammonia) (motif: Kaiser Wilhelm Bridge, Wilhelmshaven/Germany)
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Figure 20.
Azo dye with 2,2'-dihydroxy-substituted azo compound
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Figure 21.
Diazotype with ammonia under triazene formation (motif: Brandenburg Gate, Berlin/Germany)
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