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From
Monitoring pH Using Alizarin-modified Commercial Screen-printed Electrodes
Achim Habekost
World Journal of Chemical Education
.
2020
, 8(4), 163-169 doi:10.12691/wjce-8-4-4
Figure 1
.
Redox of the anthraquinone moiety
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Figure 2
.
Redox of the catechol moiety
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Figure 3
.
Schematic representation of the alizarin-modified pyrolytic graphite
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Figure 4
.
a: Reversible oxidation of alizarin: 2-electron, 2-proton process, b: Nucleophilic attack by water followed by further oxidation and tautomerism [6]
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Figure 5
.
CV of alizarin (DRP 110ALI unmodified) and MWCNT-SPE with alizarin / Nafion modified with Nafion). Dotted line: Sampling rate 0.02 V/s, unmodified DRP 110ALI-SPE. Black solid line: Scan rate 0.02 V/s, MWCNT/alizarin/Nafion-SPE. Dashed line: scan rate 0.2 V/s MWCNT/alizarin/Nafion-SPE (see the different current scales). Numbers refer to the above reaction scheme. The star symbolizes the reaction product of the dicarbonyl, see reaction (2). Wide arrow: scan direction
Full size figure and legend
Figure 6
.
pH dependence of MWCNT/alizarin/Nafion-SPE. Solid line: pH 7; dashed line: pH 4; dotted line: pH 1. Numbers refer to the above reaction scheme. The arrows indicate the two oxidation reactions (1) and (2)
Full size figure and legend
Figure 7
.
Comparison of unmodified DRP 110 ALI (dotted line) and modified DRP 110 ALI with less (solid line) and more alizarin (dashed line). Scan rate: 0.05 V/s
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Figure 8
.
Ratio between cathodic and anodic current peaks. Black: scan rate 0.05 V/s; dotted: scan rate 0.5 V/s
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Figure 9
.
pH dependence of the oxidation potential: E
p
= -58 mV/pH + 0,8 V
Full size figure and legend
Figure 10
.
Anodic current peaks as a function of pH. Arrow indicates increasing pH. Insert: Current peak at pH 11. Electrochemical method SWV
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Figure 11
.
pH dependence of the oxidation potential: E
p
= -64 mV/pH + 0,77 V
Full size figure and legend
Figure 1
2.
CV recorded twenty times in a row (black lines). After one week, the same SPE was used for the same procedure (red lines). Scan rate 0.05 V/s
Full size figure and legend