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From
Vanadium Redox Flow Batteries with Different Electrodes and Membranes
A. Habekost
World Journal of Chemical Education
.
2018
, 6(1), 8-13 doi:10.12691/wjce-6-1-2
Figure
1
. Schematic of a redox flow battery. The redox couple solutions are circulated through the redox cell containing the electrodes and the proton exchange membrane
Full size figure and legend
Figure
2
.
Components of a VRFB cell stack
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Figure 3
.
Carbon felt
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Figure 4
.
CV of vanadium (III) (left) and vanadium (IV) on graphite (right). The absence of the anodic (Figure 4, left) and cathodic current peak (Figure 4, right) indicates that the reduction V(III) → V(II) and the oxidation V(IV) → V(V) are irreversible on graphite. Scan rate 50 mV/s
Full size figure and legend
Figure 5
.
CV of vanadium (IV) on gold (Au-BT). The small cathodic current peak indicates that the oxidation V(IV) → V(V) is irreversible. Note that the cathodic peak at 0.5 V results from the sulphuric acid
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Figure
6
.
Carbon nanotubes, decorated with nano gold (SEM kindly from DropSens)
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Figure 7
.
CV vanadium (IV) at different treated carbon nanotubes. The anodic peaks around 0 V result from C=O and C-O moieties on the CNT-electrode
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Figure 8
.
Solid line: ECL of [Ru(bpy)
3
]
2+
alone (100μmol/L) , dotted line [Ru(bpy)
3
]
2+
with 30 μmol/L V(IV)
Full size figure and legend
Figure 9
.
Absorbance at 390 nm as a function of the voltage (SPE: Au-At)
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Figure 10
.
Absorbance of the oxidation product of V
4+
at different wavelengths as a function of the applied voltage. Insert: Absorption spectra derived from the absorbance vs voltage curves
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Figure 11
.
Experimental setup VRFB. From left to right: Pumps, reservoirs for the vanadium solutions, cell (between the pumps), power supply for charging, motor and data logging
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Figure 12
.
One part of the used cell with two hoses, the metal pick-up electrode and the carbon felt electrode. All compounds are mounted in a Plexiglas chamber. The alligator clip is connected with the data logging system
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Figure 13
.
Charging and discharging of a VRFB. A. Charging, B: open-circuit, C: with a motor as load
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Figure 14
.
Simple setup that shows the color change of the anode region after charging and discharging
Full size figure and legend