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From
Electrochromism of Methylviologen (Paraquat)
N. Aristov, A. Habekost
World Journal of Chemical Education
.
2015
, 3(4), 82-86 doi:10.12691/wjce-3-4-1
Fig
ure
1.
Reaction cell with incandescent lamp (left) and luxmeter (right)
Full size figure and legend
Fig
ure
2.
N-methyl viologen CV at different scan rates (50, 100, 300 mV/s) on Pt electrodes. The arrow shows the direction of scan rate increase. The bold curve shows the CV measured at 50 mV/s but only between -0.5 V and -1.0 V
Full size figure and legend
Fig
ure
3.
Total light transmission as a function of applied linearly increasing/decreasing voltage between 0 and -1.5 V and back to 0 V.
Full size figure and legend
Fig
ure
4.
A single cycle taken from Figure 3. The dashed vertical line marks the voltage turning point at -1.5 V (90 s). The solid vertical lines mark the onsets (from left to right) of reactions 1 (colorless to blue), 2 (blue to yellow), 3 (yellow to blue), and 6 (blue to colorless). The novice might need to be alerted to the fact that the potentials at which the color changes start to happen do not correspond to the peak-current potentials in the CV. The CV peak-current potentials show at which potential the reactions are most efficient, not the ones at which they can start to occur
Full size figure and legend
Fig
ure
5.
UV/vis-spectrum of viologen, measured eight times at 20-second intervals, with an applied potential of -0.9 V
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Fig
ure
6.
Total light transmission (solid curves) and measured voltage (dashed curves) of an FTO/Vio/FTO cell.
Top
: Applied voltage is -0.9 V starting at 8 s to about 25 s, then switch off of voltage to 0 V.
Bottom
: Applied voltage is 0 V up to 180 s, then electrolysis at -1.5 V between ~180 s and ~200 s, then switch off of electrolysis potential back to 0 V. At the electrolysis voltage of -0.9 V in the top panel viologen neutrals cannot form; but they can in the bottom panel
Full size figure and legend